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DOE-STD-1128-98
Guide of Good Practices for Occupational Radiological Protection in Plutonium Facilities
respiratory regions and swallowed, thereby delivering little radiation dose to the
lung tissues. Because plutonium is poorly absorbed in the gut, very little dose is
attributed to the larger particles that are cleared from the body by this process.
Small particles are deposited deeper in the lung and are cleared very slowly,
producing a much larger dose per unit activity inhaled. Extremely small particles
tend to be exhaled and not deposited.
Isotopic mixture. Characterization of the isotopic mixture is important to the
accuracy of both dose calculations and contamination measurements. When the
inventory or quantity released is expressed as the total activity (Ci or Bq) of a
mixture of isotopes, the total often includes the 241Pu activity. Because 241Pu
decays almost exclusively by beta emission, it contributes little to the internal dose
from a mixture of Pu isotopes. Also, the fraction of 241Am (from decay of 241Pu) in
plutonium can vary greatly, depending on the degree of irradiation and the time
since the plutonium was chemically separated from the reactor fuel.
Characterization of contamination from a plutonium mixture is often done by
detecting the low-energy photons emitted by 241Am, which requires knowledge of
the activity of 241Am compared to the other isotopes in the mixture.
(d) Developing Event Scenarios. The properties of the hazardous material do not
significantly affect the manner in which this step of the hazards assessment is
performed.
(e) Estimating Potential Event Consequences. For the scenarios developed in the
previous step, this step determines the area potentially affected, the need for protective
actions, and the time available to take those actions. The way these consequences are
determined depend on properties of the hazardous material.
For plutonium and its compounds, inhalation during plume passage is the most
important exposure process in the early phase of an emergency. After passage of
a plume, exposure to material deposited on the ground will dominate. Therefore,
the following features should be considered when selecting and applying
calculational models:
Inhalation pathway dose. For any realistic mixture of plutonium isotopes, the great
majority of the dose will be by the inhalation pathway. Therefore, the model
selected to estimate consequences of an atmospheric plutonium release must be
able to calculate the total effective dose equivalent (TEDE) to an individual
exposed by inhalation.
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